Hexaphenylphenylene dendronised pyrenylamines for efficient organic light-emitting diodes

Author: Thomas, K.R.J.; Velusamy, M.; Lin, J.T.; Chuen, C.H.; Tao, Y.-T.

Description: A series of blue-emitting triarylamines containing pyrene and hexaphenylbenzene dendrons were successfully synthesized by employing the Diels–Alder and palladium catalyzed C–N coupling reactions. They display high glass transition temperatures (>140 °C) in differential scanning calorimetry and facile reversible oxidation couple in cyclic voltammetry. They are also thermally stable exhibiting decomposition temperature above 385 °C. Efficient blue-emitting electroluminescent devices were fabricated using these novel amines as the hole transporting layer and 1,3,5-tris(N-phenylbenzimidazol-2-yl)benzene (TPBI) as the electron transporting layer. Colour mixing or green emission was observed when tris(8-hydroxyquinoline)aluminium (Alq3) was used as the electron transporting layer. However insertion of a thin layer of TPBI or 1,3,5-tris(4-tert-butylphenyl-1,3,4-oxadiazolyl)benzene (TPOB) in between the HTL and Alq3 layers led to pure blue emission owing to the confinement of recombination inside the HTL layer containing the compounds.

Subject headings:

Publication year: 2005

Journal or book title: Journal of Materials Chemistry

Volume: 15

Issue: 41

Pages: 4453

Find the full text : https://pubs.rsc.org/en/content/articlehtml/2005/jm/b509325b

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Type: Journal Article

Serial number: 1826